Multichannel quantum defect calculation of the phase lag in the coherent control of HI

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DOIResolve DOI: http://doi.org/10.1063/1.1370081
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TypeArticle
Journal titleThe Journal Of Chemical Physics
Volume114
Issue21
Pages94029407; # of pages: 6
Subjecthydrogen compounds; molecule-photon collisions; photodissociation; photoionisation
AbstractMultichannel quantum defect theory (MQDT) is applied within a unified framework to compute the ionization and dissociation channel phases of HI. Our numerical results illustrate the mathematical origin of a channel phase within the MQDT formalism, and are consistent with the existing theory of this phenomenon, based on the collision formalism and with experimental measurements. The present study explains why previous MQDT calculations predicted that the channel phase vanishes identically.
Publication date
LanguageEnglish
AffiliationNational Research Council Canada; NRC Steacie Institute for Molecular Sciences
Peer reviewedNo
NPARC number12328845
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Record identifier0bfd9efa-13cb-4802-93f5-83bfc9e47128
Record created2009-09-10
Record modified2016-05-09
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