Time-resolved photoelectron angular distributions as a probe of coupled polyatomic dynamics

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DOIResolve DOI: http://doi.org/10.1103/PhysRevA.64.042504
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TypeArticle
Journal titlePhysical Review A
Volume64
Issue4
Article number042504
Pages# of pages: 18
AbstractA nonperturbative theory for calculating time-resolved photoelectron angular distributions in linear molecules [J. Chem. Phys. 107, 7859 (1997)] is extended to nonlinear systems and reformulated so as to expose and utilize the underlying electronic and rotational symmetries. A sequence of approximations is next introduced, systematically reducing the formally exact expression to cruder forms that are applicable to systems of increasing complexity. As an example of the potential applications of time-resolved photoelectron angular distributions in polyatomic dynamics we examine the information they convey about an ultrafast internal conversion.
Publication date
LanguageEnglish
AffiliationNational Research Council Canada; NRC Steacie Institute for Molecular Sciences
Peer reviewedNo
NPARC number12338628
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Record identifier3ff995cd-7928-47ab-9014-e10c1430c54b
Record created2009-09-10
Record modified2016-05-09
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