Role of electron localization in intense-field molecular ionization

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DOIResolve DOI: http://doi.org/10.1103/PhysRevLett.75.2819
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TypeArticle
Journal titlePhysical Review Letters
ISSN0031-9007
Volume75
Issue15
Pages28192822; # of pages: 4
AbstractThe rate of nonlinear ionization is strongly enhanced as a molecule is stretched beyond its equilibrium internuclear separation, reaching a peak rate that is many orders of magnitude greater than that at either small or large distances. The enhancement results from nonadiabatic electron localization near the nuclei and its presence is insensitive to the laser frequency and intensity. Most intense-field dissociative ionization experiments are influenced by this effect.
Publication date
LanguageEnglish
AffiliationNRC Steacie Institute for Molecular Sciences; National Research Council Canada
Peer reviewedYes
NPARC number21276192
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Record identifier43a4d600-6938-4306-bf3c-37a7e8663347
Record created2015-09-28
Record modified2016-05-09
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