Towards disentangling coupled electronic-vibrational dynamics in ultrafast non-adiabatic processes

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DOIResolve DOI: http://doi.org/10.1039/b001138j
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TypeArticle
Journal titleFaraday Discussions
Volume115
Pages3348; # of pages: 16
AbstractFemtosecond time-resolved photoelectron spectroscopy is emerging as a new technique for investigating polyatomic excited state dynamics. Due to the sensitivity of photoelectron spectroscopy to both electronic configurations and vibrational dynamics, it is well suited to the study of non-adiabatic processes such as internal conversion, which often occur on sub-picosecond time scales. We discuss the technical requirements for such experiments, including lasers systems, energy- and angle-resolved photoelectron spectrometers and new detectors for coincidence experiments. We present a few examples of these methods applied to problems in diatomic wavepacket dynamics and ultrafast non-adiabatic processes in polyatomic molecules.
Publication date
PublisherRoyal Society of Chemistry
LanguageEnglish
AffiliationNational Research Council Canada; NRC Steacie Institute for Molecular Sciences; Security and Disruptive Technologies
Peer reviewedYes
NPARC number12327457
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Record identifiera4759dfd-03d8-4fbd-b0b9-0f76620ff098
Record created2009-09-10
Record modified2016-05-09
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