Theory of time-resolved photoelectron imaging: nonperturbative calculation for an internally converting polyatomic molecule

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DOIResolve DOI: http://doi.org/10.1103/PhysRevLett.89.233002
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TypeArticle
Journal titlePhysical Review Letters
Volume89
Issue23
Article number233002
Pages# of pages: 4
AbstractWe present the first calculation of time-resolved photoelectron angular distributions for a polyatomic system. Our method takes rotations into exact account, treats the laser field nonperturbatively, and computes the electronic dynamics from first principles. Our results point to the information content of time-resolved photoelectron imaging observables and illustrate the role played by the field intensity.
Publication date
LanguageEnglish
AffiliationNational Research Council Canada; NRC Steacie Institute for Molecular Sciences
Peer reviewedNo
NPARC number12327042
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Record identifierd14d0ece-6db9-4614-b454-e3595f6f4bbf
Record created2009-09-10
Record modified2016-05-09
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