Transient anisotropy in degenerate systems: a semi-classical approach

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DOIResolve DOI: http://doi.org/10.1524/zpch.2011.0133
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TypeArticle
Journal titleInternational Journal of Research in Physical Chemistry and Chemical Physics
Zeitschrift für Physikalische Chemie
ISSN0942-9352
Volume225
Issue9-10
Pages927938; # of pages: 12
AbstractA semi-classical model for transient anisotropy in degenerate excited states is developed on the basis of a more general ansatz presented recently [3]. This is the first model that can treat both rotational dephasing and the dynamics in degenerate systems, which is a prerequisite for a comprehensive theory to describe gas phase anisotropy experiments in small, highly symmetric systems. In the present contribution, it is shown that this model covers most of the features of the full quantum dynamical treatment and helps to give insights into the physical processes that are underlying these dynamics. © by Oldenbourg Wissenschaftsverlag, München.
Publication date
LanguageEnglish
AffiliationNational Research Council Canada (NRC-CNRC); NRC Steacie Institute for Molecular Sciences
Peer reviewedYes
NPARC number21271997
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Record identifiere8bc8796-b8e0-4199-8b39-33ea669e92c3
Record created2014-05-16
Record modified2017-03-23
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