Methods and applications of femtosecond time-resolved photoelectron spectroscopy

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DOIResolve DOI: http://doi.org/10.1016/S0368-2048(00)00212-7
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TypeArticle
Journal titleJournal of Electron Spectroscopy and Related Phenomena
Volume112
Issue1-3
Pages183198; # of pages: 16
SubjectCoincidence; Dynamics; Femtosecond; Non-adiabatic; Photoelectron
AbstractFemtosecond time-resolved photoelectron spectroscopy is emerging as a new technique for investigating polyatomic excited state dynamics. Due to the sensitivity of photoelectron spectroscopy to both electronic configurations and vibrational dynamics, it is well suited to the study of ultrafast non-adiabatic processes such as internal conversion, often occurring on sub-picosecond time scales. We discuss technical requirements for such experiments, including laser systems, energy and angle resolved photoelectron spectrometers and new detectors for coincidence experiments. We illustrate these methods with examples from diatomic wavepacket dynamics and ultrafast non-adiabatic processes in polyatomic molecules.
Publication date
PublisherElsevier
LanguageEnglish
AffiliationNational Research Council Canada; NRC Steacie Institute for Molecular Sciences; Security and Disruptive Technologies
Peer reviewedYes
NPARC number12339297
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Record identifierfa8392ad-ca41-453d-8a70-1be32f2e9bf2
Record created2009-09-11
Record modified2016-05-09
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